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Physica B: Condensed Matter, Vol. 289-290 (1-4) (2000) pp. 145-148
© 2000 Elsevier Science B.V. All rights reserved.
PII: S0921-4526(00)00300-8

Very low-temperature muon relaxation in an organic spin-Peierls compound

B.W. Lovett a * b.lovett1@physics.ox.ac.uk, S.J. Blundell a, F.L. Pratt a,b, Th. Jestädt a, W. Hayes a, S. Tagaki c and M. Kurmoo d

a Department of Physics, Clarendon Laboratory, University of Oxford, Parks Road, Oxford, OX1 3PU, UK
b RIKEN-RAL, Rutherford Appleton Laboratory, Chilton, Didcot OX11 0QX, UK
c Department of Physics, Kyushu Institute of Technology, Tobata, Kitakyushu 804, Japan
d IPCMS, 23 rue du Loess, BP 20/CR, 67037 Strasbourg Cedex, France

Abstract

We have observed strong muon-spin relaxation (µSR) in the spin-Peierls compound MEM(TCNQ)2 at temperatures down to 39 mK. We attribute this relaxation to the creation of defect spins by the muon. Furthermore, we observe a slowing down of spin fluctuations as the spin-Peierls energy gap opens, and we relate this effect to the size of the energy gap.

Keywords: Spin-Peierls; Polaron; Relaxation

*Corresponding author. Fax: +44-1865-272-400

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